Jena - I am also in Indiana and had a loan with them. Indiana payday loan laws state that the maximum allowable interest/finance charges on a payday loan are $35 ($15 on the first $100 borrowed, $10 for each additional $100), so you were only legally obligated to pay back $225, which you definitely have done.
I would send them a letter informing them that you account has been closed and they will no longer be able to debit it. I would also state that you are requesting that they mark your account as "paid in full" because you have paid $490 on a $200 loan, and according to the payday lending laws of the state you reside in, they have charged you an illegal interest rate/finance charge, and you have also been made aware that they are not licensed in the state of Indiana.
State that if they are not willing to mark your account as "paid in full", you are prepared to file complaints with the Nevada BBB, Indiana Attorney General's Office and the Indiana Dept. of Finance so they can follow up on the matter.
Send the letter to them via certified mail, return receipt requested so you have proof that it was received.